1. Introduction
High-speed information processing drives the information age. Along with the ever-increasing demand for data capacity and processing speed, photonic technologies have become a fast-evolving frontier with growing interdisciplinary interest [
1], facilitating advances in a variety of fields such as optical communications [
2], ultrafast computing [
3], precision measurements [
4], artificial intelligence [
5], and quantum optics [
6]. With a sequence of equidistant laser frequencies that are able to link the optical and electrical domain, laser frequency combs (LFCs) provide a key technology to, for example, achieve the most accurate time references to date [
7,
8], underpinning many technical breakthroughs in science and industry [
9].
Since their first experimental demonstration in 2007 [
10], LFCs generated by compact microresonators, or so-called “optical microcombs”, have become an exceptionally active research field drawing enormous attention [
11,
12,
13]. Compared to conventional LFCs generated by mode-locked solid-state or fiber lasers [
14,
15,
16], optical microcombs feature a small device volume and high compatibility for on-chip integration, which make them powerful alternatives of LFCs with reduced size, weight, and power consumption (SWaP). In addition, the repetition rates of optical microcombs, which typically range from gigahertz to terahertz and are well beyond what conventional LFCs can possibly offer [
17], intrinsically enable optical microcombs to address a range of applications that deal with high-bandwidth electrical signals, which have close connections with many core industries such as telecommunications, information processing, precision measurements, and artificial intelligence.
In tandem with the significant research on optical microcombs themselves over the past decade, there have been enormous advances in their applications in terms of both classical and quantum optics, with new applications being continually reported. As shown in
Figure 1, the applications of optical microcombs can be divided into five main categories ‒ microwave photonics, optical communications, precision measurements, neuromorphic computing, and quantum optics. The applications to microwave photonics refers to the use of optical microcombs to achieve signal handling in microwave photonic systems [
18], where microwave signals are up-converted into the optical domain, and then pass through optical modules before being down-converted back to the microwave domain. The optical communications applications represent the realization of high-speed data transmission based on optical microcombs, with high-speed electrical signals being modulated onto optical microcombs that serve as sources of multiple optical carriers. Precision measurements include the use of optical microcombs to achieve measurement functions such as spectrum analysis, ranging, and frequency measurements. The neuromorphic computing applications include the use of optical microcombs to realize different computing functions in neuromorphic systems, which take inspiration from biological visual cortex systems to create power-efficient computing hardware that is capable of handling sophisticated tasks [
19]. Quantum optics based on microcombs provide novel quantum optical sources for quantum information science, mainly involving the generation of single photons, entangled photons, and squeezed light [
6].
The chronology for the applications of optical microcombs is shown in
Figure 2(a).
Figure 2(b) shows the number of relevant publications in Science Citation Index (SCI) journals versus year since 2012. Both of these highlight the rapid growth in the use of optical microcombs for different applications, which has been driven mainly by three factors. First, the performance of optical microcombs has been continually improving in terms of its spectral bandwidth, energy efficiency, phase coherence, and stability, and this has significantly enhanced their performance in these applications. Secondly, optical microcombs have become more widely used for traditional and demanding applications, such as frequency synthesis [
20,
21,
22,
23,
24,
25,
26,
27,
28], spectral filtering [
29,
30,
31,
32,
33], temporal signal processing [
34,
35,
36,
37,
38,
39,
40], and optical communications [
33,
41,
42,
43,
44,
45]. Finally, many new and exciting interdisciplinary applications have emerged, spanning the frontiers of light detection and ranging (LiDAR) [
46,
47,
48,
49], astronomical detection [
50,
51,
52,
53], neuromorphic computing [
54,
55,
56], and quantum optics [
11,
57,
58], which bring significant new opportunities.
In this paper, we review the applications of optical microcombs, including microwave photonics, optical communications, precision measurements, neuromorphic computing, and quantum optics. While optical microcombs have been the subject of recent reviews [
9,
11,
12,
13,
61,
62], they have predominantly focused on the physics or dynamics of the optical microcombs themselves, rather than their applications. In addition to reviewing the state-of-the-art of these fields, we provide quantitative analysis for the key performance parameters for some of the most important applications. We also highlight the open challenges and future directions for both conventional and emerging applications.
This paper is structured as follows. In
Section 2, we review the advances in generating optical microcombs, being categorized into material platforms, device architectures, soliton classes, and driving mechanisms. Next, the applications of optical microcombs to microwave photonics are discussed in
Section 3, including frequency synthesizers, microwave photonic filters, and microwave photonic signal processors. In
Section 4, the use of optical microcombs for optical communications in both coherent and intensity modulation - direct detection (IM -DD) transmission systems is reviewed. In
Section 5, precision measurements based on optical microcombs are reviewed, including dual-comb spectroscopy, ranging, astrocombs, frequency measurements, and spectrum channelizers. In
Section 6, neuromorphic computing applications of optical microcombs are reviewed, including those in both single neurons and neural networks. The applications of quantum microcombs are summarized in
Section 7, including the generation of single / entangled photons and squeezed light. The current challenges and future perspectives are discussed in
Section 8. Finally, conclusions are given in
Section 9.
8. Challenges and Perspectives
The past decade has witnessed rapid growth in research on optical microcombs, including the improvement of their performance as well as expansion of their range of applications. As evidenced by the substantial body of work reviewed in previous sections, the applications of optical microcombs have rapidly expanded and achieved considerable progress ‒ in both traditional and emerging new applications. Despite this remarkable success, though, there are still open challenges and limitations that need to be addressed. In this section, we discuss these in terms of both research and industrial applications.
Paralleling the development of micro / nano fabrication technologies, the family of material platforms for generating optical microcombs has grown substantially.
Figure 26 compares the state-of-the-art of the different material platforms. For optical microcomb generation, a high Kerr nonlinearity to improve the conversion efficiency, a large bandgap to reduce the TPA, and a high Q factor with reduced linear loss are key goals. As shown in
Figure 26(a), materials with high Kerr nonlinearities (
i.e.,
n2) tend to have lower bandgaps [
83,
91,
92,
95]. Similarly, there is also a trade-off between achieving a high Q factor versus a high Kerr nonlinearity, as shown in
Figure 26(b), since higher refractive index materials yield larger nonlinearities, but on the other hand also tend to produce higher waveguide loss, and hence lower Q factors. These trade-offs need to be considered and properly balanced in developing new material platforms for optical microcomb generation. Amongst the various optical microcomb platforms, CMOS-compatible platforms such as Si
3N
4, Hydex, SiC, SiO
2, and Ta
2O
5, are promising to facilitate large-scale manufacturing of commercial devices. Some platforms, such as Si
3N
4, LiNbO
3, GaP, and AlGaAs, that can be co-integrated with other functional components on chips such as lasers, EO modulators, and PDs, are attractive for implementing monolithically integrated systems.
Figure 26(c) compares the FSRs of microresonators based on different material platforms, which are plotted in the microwave frequency band (0.3 GHz ‒ 300 GHz) given that it has close relations with the majority of state-of-the-art applications of optical microcombs. Before 2010, microcombs with small FSRs of less than 100 GHz were mainly generated by discrete and often bulk based WGM cavities such as toroids, wedged disks, and rod resonators [
65,
71,
142]. By virtue of the advances in integration fabrication technologies in the past decade, many fully integrated MRRs with much smaller FSRs can now generate microcombs. This is highlighted by micro-combs generated by Si
3N
4 MRRs with FSRs down to 10 GHz [
26], Hydex MRRs with FSRs down to 49 GHz [
30], and LiNbO
3 MRRs with FSRs down to 10 GHz [
93]. In addition, recent progress in the on-chip integration of WGM microcavities [
138] opens up a new avenue for generating small-FSR optical microcombs based on photonic integrated chips.
Achieving reliable and self-starting mode locking are both critical capabilities needed to enable stable and coherent optical microcombs for many applications such as frequency synthesizers, optical communications, and precision measurements. As reviewed in
Section 2.4, in recent years, many new mode-locking approaches such as cryogenic cooling [
88], auxiliary laser heating [
159], and nonlinear dynamics engineering [
110] have been proposed, and conventional mode-locking approaches such as self-injection locking and filter-driven four-wave mixing have also experienced new developments [
106,
334]. For practical applications, there are two main directions for improvement. One is achieving easy-to-operate mode-locking without complex startup processes, recently demonstrated with turnkey soliton microcomb generation [
110], offering the promise of further improving the system stability and control of the feedback phases. The other direction involves realizing on-chip mode-locking systems, where, for example, the piezoelectric control of microcombs via integrated actuators and the portable battery-operated soliton microcomb generator have represented significant advances. Alternative approaches may involve the use of 2D materials with strong saturable absorption to enable simple passive mode locking, as has been demonstrated in mode-locked fiber lasers [
335,
336].
Microcomb-based frequency synthesizers have been used for synthesizing not only microwave but also optical frequencies ‒ well beyond that offered by LFCs generated from solid-state lasers and mode-locked fiber lasers [
16,
206,
207]. Although the frequency stability and spectral purity of microcomb-based frequency synthesizers are still not as good as their bulky counterparts, the gap between them is continuously narrowing owing to the advances in technologies for generating soliton microcombs with high coherence and stability [
88,
159,
192]. By further reducing the linewidths and noise of lasers for pumping microcombs as well as improving the mechanical and thermal stability of microcomb-based frequency synthesizing systems, there is still room for future improvement. In addition, compared with direct generation of microwave frequencies via photodetection, frequency synthesizers based on optical-to-microwave frequency division normally show higher purity and better frequency stability. As a result, they are preferable for demanding applications with more stringent requirements for frequency deviation and noise performance.
For microcomb-based microwave photonic filters, the filtering resolution has been significantly improved by using microcomb sources with smaller FSRs to provide increased numbers of wavelength channels or taps,
e.g., a Hydex MRR with an FSR of ~49 GHz that provides 80 wavelength channels in the C-band [
30]. To increase the resolution further, more available wavelength channels can be obtained by using MRRs with even smaller FSRs down to ~10 GHz [
26], but this comes at the expense of reduced FSRs in the RF response spectra. Another option is to extend the operation band, for example, into the L band (1570 ‒ 1620 nm). This requires some specialized L-band components in the transversal filter system such as EO modulators, wave shapers, and PDs to be upgraded with broader operation bandwidths. Out-of-band rejection is another critical parameter for microwave photonic filters, which can also be improved by increasing the tap numbers in the microwave photonic transversal filters. In addition, although Gaussian apodization has been applied to improve the out-of-band rejections [
30], it also results in degraded filter resolution, reflecting the trade-off between these two parameters for a fixed tap number.
For microcomb-based microwave photonic signal processors, basic analog signal computing functions, such as (either integral or fractional-order) differentiation [
37,
224], integration [
38], and (either integral or fractional-order) Hilbert transform [
34,
35], have already been realized based on transversal filter systems. More complex functions, such as high-order integration and solving differential equations [
235,
337,
338,
339], are expected to be achieved by designing the corresponding tap coefficients. State-of-the-art microwave photonic signal processors based on microcombs show higher processing accuracy than what can be achieved by directly processing optical analog signals using passive optical devices [
232,
233,
340], although their accuracy is still not as high as their electronic counterparts. In practical systems, there are a number of factors that lead to processing inaccuracy.
Figure 27(a) shows a typical microcomb-based transversal filter system, where the error sources mainly include (I) a limited number of taps, (II) phase noise of the microcombs, (III) uneven gain and noise of the optical amplifiers, (IV) time delay and shaping inaccuracy caused by optical spectral shapers, (V) chirp of the electro-optic modulators (EOM), (VI) high-order dispersion of the dispersive fiber, and (VII) noise of PDs. Amongst them, the errors induced by (I) can be reduced by using resonators with smaller FSRs or optical amplifiers with broader operation bandwidths. (II) can be lowered by using a range of mode-locking technologies as mentioned previously. The errors arising from (III) ‒ (VI) can be compensated for by using feedback control circuits to calibrate the system impulse response. By using a two-stage comb shaping strategy [
38], the inaccuracy induced by (III) and (IV) can also be improved. (VII) can be reduced by employing balanced PD to eliminate the common mode noise.
Monolithic integration is a key issue that has experienced significant recent development. It is critical for future microwave photonic filters and signal processors based on optical microcombs. Although just using integrated microcomb sources to replace discrete laser arrays already yields significant benefits in terms of SWaP, cost, and complexity, there is much more to be gained by increasing the level of integration for the overall system.
Figure 27(b) shows the concept of a monolithically integrated transversal filter system with a microcomb source, which includes a CW laser, an MRR, an optical amplifier, an EOM, an optical spectral shaping array, a delay element array, and a PD. Compared with the system in
Figure 27(a), the SWaP are greatly reduced, reaching the chip scale. In principle, all the components in
Figure 27(b) can be integrated on the same chip. For instance, InP/Si semiconductor lasers and Si
3N
4 MRRs have been heterogeneously integrated to generate soliton microcombs [
135]. Semiconductor optical amplifiers (SOAs) [
341], Si or InP spectral shapers [
342,
343], LiNbO
3 modulators [
344], delay lines [
345], and Ge PDs [
346] have also been demonstrated in integrated forms. Recently, some submodules of the system have already been realized, such as the microcomb source chip consists of heterogeneously integrated pump lasers and microresonators [
136], and the processing chip contains modulators, shaping arrays, and delay lines [
33]. All of these pave the way for implementing the whole system on a single chip in the future.
For coherent optical communications based on microcombs, the state-of-the-art data rate and SE have reached over 50 Tbit/s [
42] and 10 bits/s/Hz [
43], respectively, using high-order modulation format up to 256-QAM [
43,
44]. To improve the data rate and SE, even higher-order modulation formats as well as other multiplexing methods such as poly polarization or orbital angular momentum multiplexing can be employed [
347,
348], although these would also bring more stringent requirements for the OSNR and the BER. Emerging mode-locking technologies, such as auxiliary laser heating [
159] and turnkey soliton microcomb generation [
110], can be applied to improve the comb stability and simplify the operation of these systems. In addition, in demonstrations of coherent communications reported to date based on microcombs, most of the components in the transmitters and receivers other than the microcombs have been discrete devices. Similar to the microcomb-based signal processors in
Figure 27(b), monolithically integrated transmitters and receivers with significantly reduced SWaP will be the subject of future research. For IM-DD optical communications, PAM8 or even higher modulation formats can be used to further increase the data rate on the basis of state-of-the-art PAM4 systems. This also requires a higher OSNR of the comb lines, which can be achieved through modifying the device architecture or employing soliton crystals, dark solitons, or laser cavity solitons that have high conversion efficiencies. In addition, the quantum characteristics of optical microcombs could be exploited for realizing secured communications with unprecedented capability [
57].
For precision measurements based on optical microcombs, in addition to conventional spectroscopy, many other functions have been demonstrated such as ranging [
46,
48], measurements of Doppler shift and frequency [
52,
143]. Compared with LFCs generated by mode-locked fiber lasers, optical microcombs feature larger repetition rates, which enables low acquisition time and broadband sampling of optical spectra, but at the same time results in relatively low resolution. To achieve higher resolution, channelizers can be employed to slice the spectra of broadband microwave signals into small-bandwidth segments. As reviewed in
Section 5.5, the state-of-the-art microcomb-based microwave spectrum channelizers already achieve a 100-MHz-level slice resolution [
271], which is compatible with the real-time bandwidths of electronic devices. In the future, portable or even monolithically integrated sensors based on DCSs are expected to be achieved, with expanded applications in fields such as medical diagnosis, exoplanet analysis, combustion studies, biological tests, meteorology observation, and bio-chemical threat detection. New measurement functions are also expected to enable the characterization of other parameters, such as time-frequency distribution, angle-to-arrival, and noise. In addition, microcomb-based precision measurements can be applied to more complex microwave photonic radar systems, where there has already been encouraging preliminary work [
212,
217].
For applications to neuromorphic computing, single neurons and simple CNNs with a single hidden layer have been realized based on vector operations such as dot product and convolution. The microcomb-based CNNs have achieved processing speeds that are far superior to their electronic counterparts [
56], but the accuracies have not reached the same level. Aside from the previously mentioned methods for improving the computing accuracy of microwave photonic signal processors, the recognition accuracy can be improved further by increasing the scale of the fully connected layers [
56]. On the other hand, the existing CNN systems can be scaled to realize deep CNNs with multiple hidden layers, which can accomplish more complicated tasks. Issues that need to be addressed include the performance of input / output interfaces between adjacent layers, deteriorated processing accuracy caused by increased system complexity, and synergy control among different layers. In addition, through flattening digital images into vectors, and then converting them to analog signals, digital image processing or even video processing can be realized based on optical microcombs. This offers new possibilities for realizing a wide range of image processing functions, including traditional functions such as edge enhancement and motion blur [
228,
229], as well as new computer vision applications such as autonomous vehicles, face recognition, remote drones, and medical diagnosis [
50,
51,
349].
The scale of state-of-the-art quantum systems based on optical microcombs can be further expanded by using microresonators with smaller FSRs as well as integrated EO modulation and spectral phase manipulation schemes [
342,
350]. To achieve this, broadband detection techniques for frequency-encoded photon states will also be needed [
351]. Deterministic sources are critical for implementing efficient quantum systems. Similar to other sources based on the spontaneous nonlinear optical processes, optical microcombs are stochastic in nature. Therefore, the challenges for implementing deterministic microcomb-based quantum systems are similar to those of deterministic single-photon sources. Since optical microcombs are capable of providing a large quantum resource per photon, they offer new possibilities to compensate for the drawbacks of non-determinism. The miniaturization of quantum microcombs, which is crucial for practical applications, remains a technological challenge. A pulsed quantum-microcomb excitation scheme has been demonstrated recently [
352], paving the way for the realization of monolithic quantum microcombs. The continuous improvement of microcombs’ performance as well as progress in their classical applications will also naturally benefit the future advances in quantum applications of optical microcombs.
Achieving microcomb generation in the visible region, where several atomic transitions (
e.g., Rb, Hg
+, and Yb) that are being used as time references for atomic clocks are located [
189,
353], offers new possibilities for realizing miniatured optical atomic clocks, optical coherence tomography systems [
354], and visible-band mode-locked systems [
355]. The challenges here not only revolve around having to work with platforms that are low loss in these shorter wavelength regimes (
e.g., ruling out silicon) but the challenge is that it is much more difficult to engineer anomalous dispersion. Furthermore, the waveguide dimensions become significantly smaller to achieve single-mode operation. Many experimental demonstrations of visible microcomb generation have already been reported, such as those based on engineering the mode hybridization [
331], the second-order nonlinear interactions [
101,
113,
356], high-order modes [
111], and the Cherenkov-like radiation [
357]. However, most have only managed to generate microcombs above 700 nm, at the boundary between the visible and near IR wavelengths, hinting at more breakthroughs in generating visible microcombs at shorter visible wavelengths (< 600 nm).
Finally, there is a high degree of synergy between advances in optical microcombs and their fast-expanding areas of applications. On the one hand, optical microcombs with compact footprint, low power consumption, and large comb spacing offer enormous new possibilities for a variety of applications in both conventional and new interdisciplinary fields. On the other hand, driven by the growing requirements in practical applications, controlling and optimizing microcombs’ performance, as well as investigating the underlying physics (
e.g., imaging the DKS dynamics with a high resolution < 1 ps [
160]) become increasingly demanding, which will facilitate the rapid development and wide deployment of optical microcombs. This synergy will have a long-lasting positive impact, which will be a strong driving force for the continual improvement in performance and the broadening of its applications to deliver the promised benefits of LFCs based on photonic integrated chips. Research on the applications of optical microcombs will undoubtedly continue to thrive, in parallel with the development of relevant commercial products that will eventually enable the bridging of the gap between laboratory-based research and practical industrial applications.