1. Introduction
Diffusion is a process of spontaneous movement of particles due to collisions with other particles. These collisions can occur between diffusing particles as well as particles of the medium in which diffusion occurs. The fundamental characteristic of this type of movement is that the mean square displacement of the particle (the square of its dispersion), depends non-linearly on time [
1,
2]
as opposed to the linear dependence (
) that characterizes Brownian motion. In the first case, when the exponent of the power is less than one, it is called subdiffusion, whereas when the diffusion exponent is greater than one, it is called superdiffusion. The second case concerns the so-called Lévy flights which have been observed experimentally [
3,
4,
5]. Subdiffusion is most commonly observed in media such as gels and porous media, where particle movement is extremely difficult [
6,
7].
The thermal conductivity, which involves the flow of heat through solid substances like metal, is a twin process to diffusion. It is a process where thermal energy is transferred through conduction by the transfer of particle vibrations. The particles in a solid state are close to each other and are held together by intermolecular forces. When one particle gains energy, it transfers it to the neighboring particle through vibration transfer. Mathematical models incorporating fractional-order derivatives are excellent tools for describing thermal conduction in porous materials, such as porous aluminum [
8].
Within the framework of subdiffusion or thermal conductivity processes modeled by subdiffusion or the fractional thermal conductivity equation, a subclass of so-called fractional Stefan problems can be distinguished. They are designed to describe the evolution of the boundary between two phases of a material undergoing a phase transition. Examples include the drug release from slab matrices [
9,
10]. Numerous papers presenting analytical and numerical results have been devoted to this phenomenon [
11,
12,
13,
14,
15,
16,
17].
In the papers [
18,
19], Povstenko et al. consider the two dimensional time-fractional heat conduction equations. In the solution, they use Laplace and Fourier integral transforms, which allow the reduction of higher-degree differential equations to lower-degree equations, which greatly improved the obtaining of the solution. In addition, the paper [
19] uses the Gaver-Stehfest algorithm to invert the Laplace transform. A similar approach to those presented in the aforementioned papers is used in this article, based, moreover, on the results presented in the monograph [
20], with the difference that the Gaver-Wynn-Rho algorithm [
21,
22,
23] was used to determine the original solution from the Laplace transform image.
Numerous numerical methods have been proposed for solving equations of anomalous diffusion. Ciesielski introduced numerical schemes for various cases in his doctoral dissertation [
24], including equations with fractional-order time and spatial derivatives. The discussed cases were limited to one-dimensional problems. Papers [
25,
26] considered one-dimensional subdiffusion equations with a fractional spatial Riemann-Liouville derivative and provided corresponding numerical schemes. Bhrawy et al. [
27] presented a numerical method for a subdiffusion equation with a Caputo time derivative. Błasik [
28,
29,
30] extended the classical Crank-Nicolson method to one-dimensional subdiffusion equations with a Caputo time derivative, considering a variable diffusion coefficient and nonlinear source term. Other variants of the Crank-Nicloson method for the subdiffusion equation are included in the papers [
31,
32,
33]. Noteworthy are also the articles [
34,
35,
36,
37,
38], in which the authors have developed numerical methods characterized by high accuracy. Numerical results for the two-dimensional subdiffusion equation were presented in papers [
39,
40], while a more general case involving a source term was discussed in [
41,
42]. Other numerical approaches related to subdiffusion concern inverse problems [
43] and use a non-standard definition of the Caputo derivative [
44].
The article was structured as follows. The second section presented the basic definitions and properties of the following: fractional order differential calculus, integral transforms, and numerical methods. These concepts were utilized throughout the rest of the article. In the subsequent section, the problem to be solved was formulated as a two-dimensional sub-diffusion equation, along with uniqueness conditions. Two different methods were employed to solve this problem, each discussed in its respective sub-section. The fourth section showcased the numerical results obtained from the calculations. Finally, the article concluded with a section summarizing the findings and providing additional insights.
2. Preliminaries
Let us begin our consideration by introducing two fractional order operators: the left-sided Riemann-Liouville integral and the left-sided Caputo derivative together with the composition rule of the two mentioned operators [
45].
Definition 1.
The left-sided Riemann-Liouville integral of order α, denoted as , is given by the following formula for :
where Γ is the Euler gamma function.
Definition 2.
Let . The left-sided Caputo derivative of order α is given by the formula:
Property 1 (Lemma 2.22 in [
45]).
Let function . Then, the composition rule for the left-sided Riemann-Liouville integral and the left-sided Caputo derivative is given as follows:
The definition of the Laplace integral transform [
46], combined with the following property [
47], will play an important role in determining the semi-analytical solution of the problem considered in the next section.
Definition 3.
Let be a real function of the variable . Then the Laplace transform of the function is the function of the complex variable defined by formula
where .
Property 2.
Let the function be the original, and let , then the following formula holds
Bessel functions of the first and second kind [
45,
48] present two further definitions.
Definition 4.
Let and , then the Bessel function of the first kind denoted by is given by the following series:
Definition 5.
Let , then the Bessel function of the second kind denoted by is given by the following formula:
In the case of integer order , function is defined in terms of the limit of
The numerical scheme proposed in the next section uses a mesh of nodes defined as follows:
Definition 6. Let be a continuous region of solutions for the partial differential equation. Then the set we call the rectangular regular mesh described by the set of nodes.
In the further part of the paper, the real order of the left-sided Caputo derivative, and the left-sided Riemann-Liouville integral is considered.
3. Mathematical formulation and solution of the problem
Consider a two-dimensional subdiffusion equation in a region with axial symmetry. Let us also assume an axisymmetric system of boundary and initial conditions. The equation under consideration has the form:
supplemented by boundary conditions on the edges of the circular ring:
and initial condition
where the generalized diffusion coefficient
is constant.
In the axisymmetric region in which we derive the solution of the differential equation, it is convenient to introduce the polar coordinates given by:
,
, for which the differential Equation (
10) with boundary and initial conditions takes the form of:
The assumptions made about symmetry allow us to reduce the dimension of the problem under consideration. Let us note that for a fixed radius
r and arbitrary angle
, the diffusion flux in the direction normal to the edge takes the constant values. Thus, the function
U does not depend on
, and the second differential term on the right hand side of Equation (
14) is equal to zero. As a result, the two-dimensional equation is immediately reduced to the one-dimensional one:
It should be mentioned that in addition to symmetry, there are other ways to reduce the dimensions of differential problems, such as scaling [
49,
50], and integral transforms [
46], which will be shown in the next section.
3.1. A numerical approach
In the paper [
28], a generalized Crank-Nicolson method was proposed for the one-dimensional subdiffusion equation. The obtained results were further extended to the more general case, to the equation with a source term [
29]. In both cases, obtained results confirmed the accuracy of the proposed methods. Therefore, an analogous approach will be applied to the problem defined by equations (
18)-(
21).
For some technical reasons, the numerical approximation of the left-sided Caputo derivative is much simpler compared to the approximation of the left-sided Riemann-Liouville integral. Therefore, we apply Property 1 to the Equation (
18), which yields an integro-differential equation in the following form:
The solution
U of the initial boundary value problem considered in the paper fulfills the assumptions of Property 1, and its existence and the uniqueness was proven in the more general case in the paper [
51]. Further consideration will be conducted with reference to the mesh of nodes given in Definition 6. For each node of the grid, we determine the discrete form of the integral kernel in the integrals on the right-hand side of Equation (
22). For this purpose, we approximate the solution
U by a linear function between two consecutive nodes with respect to the variable
t:
for
,
.
Subsequently, we discretize the first- and second-order derivatives of the right-hand side of the integro-differential equation (
22) using differential quotients approximating the first
and second derivative
with respect to the spatial variable
r.
Using transformations analogous to those in the paper [
29], we obtain the discrete form of integro-differential equation (
22) as follows:
where the weights corresponding to the integral kernel of the left-sided Riemann-Liouville integrals are of the form:
We transform Equation (
26) in such a way that the unknown values of the
U function in the k-th time layer are on its left side. Finally, we obtain an implicit numerical scheme, which in node
takes the form:
Applying the above relationship to each of the
nodes of the k-th time layer, we obtain a system of linear equations with
unknown values of the
U-function, which can be written in matrix form:
where matrix
A is defined by
where
. The elements of vector
B are defined by
where
3.2. A semi-analytical approach
The application of the Laplace transform and Property 2 to subdiffusion Equation (
18) removes the time variable, thus reducing the considered equation to the form of an ordinary differential equation, which is solved in terms of the space variable
r. As a consequence of this treatment, we get the equation:
supplemented with boundary conditions
We can write the boundary value problem (
30)-(
32) as follows, using the notation for ordinary differential equations:
The differential equation (
33) is the so-called Bessel differential equation, whose general solution is well known in the form of Bessel functions of the first and second kind [
48]:
Applying the boundary conditions (
34) and (
35) to Equation (
36), we obtain a system of equations:
Solving the system of equations (
37), we obtain a constant
in the form of:
and a constant
in the form of:
Obtaining the original
by analytical transformations is problematic, therefore this task will be realized in the next section using the Gaver-Wynn-Rho algorithm [
21,
22,
23].
4. Numerical examples
The numerical results presented in the following section assume the following values for the parameters of the initial boundary value problem (
18)-(
21):
,
,
,
. Numerical simulations were performed for seventeen mesh variants, which adopted:
.
The figures shown below illustrate the results of numerical calculations, which assumed the following values of grid steps: and . This choice provides a compromise between good readability of the graphs and accuracy of the presented results.
Figure 1,
Figure 3,
Figure 5 and
Figure 7 show the solutions of the subdiffusion Equation (
18) depending on the radius
r at four different time instants. They clearly demonstrate the nature of the modeled phenomenon. For very early time instants just after the initiation of the process
, the solution obtained for
reaches the largest values. The disproportion between the solution for
and
decreases with the increase of time, and this results directly from the relation (
1).
Figure 7 shows that for
, the solution obtained for
takes the largest values.
Figure 2,
Figure 4,
Figure 6 and
Figure 8, present the axial symmetry of the obtained solutions in the Cartesian coordinate system. The values of the variable
were determined as follows:
,
. The
x,
y coordinates were determined using the relationship
,
.
Figure 1.
Plot of determined numerically for , .
Figure 1.
Plot of determined numerically for , .
Figure 2.
Plot of function .
Figure 2.
Plot of function .
Figure 3.
Plot of determined numerically for , .
Figure 3.
Plot of determined numerically for , .
Figure 4.
Plot of function .
Figure 4.
Plot of function .
Figure 5.
Plot of determined numerically for , .
Figure 5.
Plot of determined numerically for , .
Figure 6.
Plot of function .
Figure 6.
Plot of function .
Figure 7.
Plot of determined numerically for , .
Figure 7.
Plot of determined numerically for , .
Figure 8.
Plot of function .
Figure 8.
Plot of function .
In order to validate the numerical method proposed in subsection 3.1, the results obtained with it were compared with those received by the inverse Laplace transform of the image (
36) using the Gaver-Wynn-Rho algorithm implemented in Wolfram Mathematica. The comparison was made at twenty points
, which are common to all tested mesh variants.
Table 1,
Table 2,
Table 3 and
Table 4 collect the average absolute difference between the solution obtained by the proposed numerical method
and that obtained by the inverse Laplace transform
. The analysis of all the tables leads to the observation that as the steps of the grid
and
are reduced, then
converges to
for all tested values of the order
.
4.1. Convergence analysis
The order of convergence of the proposed numerical scheme was estimated using EOC (experimental order of the convergence) and calculated as follows [
35]:
where by
denoted the numerical solution of the considered equation at nodal points common to all considered meshes
for
,
, with time step
and spatial step
. By
the reference numerical solution obtained under the fine mesh is denoted. We use the formula (
40) only when the closed analytical solution is not available. The calculation results shown in
Table 5 and
Table 6 indicate that the order of convergence of the proposed method is approximately equal to one. We can come to similar conclusions by comparing the elements on the main diagonal in
Table 1,
Table 2,
Table 3 and
Table 4.
5. Conclusions
The method proposed in the article is a generalization of the fractional Crank-Nicolson method to a two-dimensional subdiffusion equation in the polar coordinate system, taking into account the assumed symmetry of the area and boundary conditions. To validate the method, the obtained results were compared with those received using the semi-analytical approach, where the analytical solution in the Laplace transform domain was numerically inverted. It was observed that the method based on the discretization of the integro-differential equation generates solutions that converge to those obtained by the Gaver-Wynn-Rho algorithm. As the time and space steps are decreased, the average absolute difference between the solutions decreases.
Furthermore, it was found that the semi-analytical approach is more effective in determining the solution at specific points within the area, despite the relatively longer time to obtaining a solution at a single point. On the other hand, the generalized Crank-Nicolson method allows for the determination of the solution at all nodal points within the area significantly faster, but with lower accuracy. In the tests, it took approximately 10 seconds to obtain solutions for 10201 nodal points, while the Gaver-Wynn-Rho algorithm generated solutions for 20 points in about 3 seconds.
In a subsequent stage of testing, the plan is to further investigate the convergence analysis of the proposed scheme and reduce the computational cost.
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Table 1.
The value of for .
Table 1.
The value of for .
Table 2.
The value of for .
Table 2.
The value of for .
Table 3.
The value of for .
Table 3.
The value of for .
Table 4.
The value of for .
Table 4.
The value of for .
Table 5.
Convergence order of the proposed numerical scheme for .
Table 5.
Convergence order of the proposed numerical scheme for .
|
= 1 |
= 0.75 |
n |
m |
|
|
|
EOC |
|
EOC |
50 |
25 |
|
|
4.721e-3 |
- |
2.759e-3 |
- |
100 |
50 |
|
|
1.781e-3 |
1.406 |
6.509e-4 |
2.084 |
200 |
100 |
|
|
7.416e-4 |
1.264 |
2.857e-4 |
1.188 |
400 |
200 |
|
|
2.939e-4 |
1.3353 |
1.231e-4 |
1.215 |
Table 6.
Convergence order of the proposed numerical scheme for .
Table 6.
Convergence order of the proposed numerical scheme for .
|
= 0.5 |
= 0.25 |
n |
m |
|
|
|
EOC |
|
EOC |
50 |
25 |
|
|
1.15e-3 |
- |
2.836e-4 |
- |
100 |
50 |
|
|
1.788e-4 |
2.684 |
7.505e-5 |
1.918 |
200 |
100 |
|
|
1.117e-4 |
0.679 |
4.03e-5 |
0.897 |
400 |
200 |
|
|
4.913e-5 |
1.186 |
1.715e-5 |
1.233 |
|
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