1. Introduction
The idea of Basov and Krokhin to fire with a laser thermonuclear (TN) reaction between deuterium and tritium (D−T) during a short time compared to the hydrodynamic expansion of heated plasma, i.e., to obtain the inertial confinement fusion (ICF) in the micro explosion [
1], is currently under a comprehensive investigation. It is either in a direct-drive irradiation of a shell target with TN fuel by laser light [
2], or in the indirect scheme with converting laser radiation into X-rays in the cylindrical capsule with a target inside [
3]. Nowadays, when the ignition of TN reaction has been already achieved in the indirect-drive at NIF Nd: glass laser facility [
4], it is quite obvious from a prolonged experimental run [
5,
6,
7,
8] that the main obstacle on the path to ignition are hydrodynamic instabilities. From initial perturbations caused by either target imperfections or X-ray irradiation asymmetry they rapidly develop into the turbulent phase during shell acceleration, as well as its deceleration afore the target collapse.
In the direct-drive scheme initial small-scale perturbations besides a roughness of the shell surface are mainly caused by speckles typical for irradiation by a coherent light. A large-scale asymmetry arises either because of a limited number of laser beams even in the advanced ICF laser facilities (e.g., about 200 for the biggest ones NIF [
9] and LMJ [
10]) or energy misbalance between the beams. The latter originates from energy exchange in a course of nonlinear laser interaction with underdense outer plasma corona [
11]. The small-scale hydrodynamic perturbations are seeded via "laser imprinting" at the very beginning of target irradiation, before plasma corona being formed: light inhomogeneities are directly transformed into inhomogeneous profile of the ablation front moving inward the shell [
12]. The growth of instabilities and their transition into the turbulence lead to mixing of the TN fuel and shell material followed by temperature and density decrease in the target core which results in a sharp fall of the TN reaction rate and prevents the TN fuel burning.
To uniform the distribution of laser radiation over a target surface, many optical methods have been developed (they are described e.g., in the review [
11]) that are random phase plates, phased zone plates, and kinoform phase plates. As well an optical smoothing was demonstrated by angular dispersion of frequency-modulated laser light, induced spatial incoherence (ISI) produced by echelons. To reduce the effect of laser imprinting, in addition to optical methods, there are various hydrodynamic methods based on the creation of a plasma layer in front of the target with a density gradient towards the target before the arrival of the main heating pulse. Such absorbing plasma with a density somewhat higher than the critical one evens out the irradiation inhomogeneities due to transverse thermal diffusion [
13]. It can be created by ionizing a gas [
14] or a porous medium, i.e., a foam with a low volume density placed in front of the plastic ablator by a low-energy prepulse [
15,
16]. A near-critical-density (NCD) preheated foam plasma can be also produced by X-ray radiation from a nearby laser-plasma source [
17,
18], or by using a thin (<1000 Å) layer of a high-Z material, which is deposited on the target surface or incorporated into the foam facing the laser [
19,
20,
21]. In the latter case, laser-heated high-Z plasma effectively re-radiates in the soft X-ray range, causing uniform ablation of the target. As a result, the distance between the absorption zone of laser radiation nearby the critical plasma density and the ablation front increases, which leads to smoothing of the laser imprint.
Laser-foam interaction including ionization dynamics of foams have been studied experimentally and theoretically in many works mostly with Nd: glass lasers at wavelength λ = 1060 nm, sometimes at second (2ω) or third (3ω) harmonics (see, for example, [
22,
23,
24,
25,
26,
27,
28,
29,
30,
31,
32,
33,
34,
35,
36,
37,
38]). It is commonly assumed that foams are initially transparent for laser radiation and plasma is originated from evaporation and ionization of pore septa. Meantime, compared with a Nd: glass laser, KrF laser looks more attractive in the role of ICF driver, and especially for the production of the Inertial Fusion Energy (IFE), as it can be scaled to required sub-megajoule pulse energy, operate with overall efficiency up to 7% at rep-rate 5−10 Hz and be arranged by a focal spot zooming synchronously with a target implosion [
39,
40]. As KrF fundamental radiation UV wavelength λ = 248 nm is one and a half times less than the 3ω Nd: glass laser, it has a number of important advantages in laser-target interaction: higher ablation pressure and efficiency of laser energy transfer into the kinetic energy of the imploding target, higher thresholds of laser-plasma instabilities (LPI) in the plasma corona and, accordingly, less amount of harmful fast “superthermal” electrons preheating the dense target core before the collapse. The effective echelon-free ISI smoothing of a broad-bandwidth radiation with a noncoherent master oscillator was implemented on Nike KrF laser facility [
41]. An overlapping of 44 noncoherent beams with a total energy about 1.7 kJ in 4-ns pulses produced on a planar target intensity
I ~ 10
14 W/cm
2 with the highest ever achieved uniformity with an rms deviation ~ 0.15% within the spot of 500−1000 μm. A stepwise laser pulse-form used in early experiments [
42,
43] and supposed for the ICF-scale target design [
44] had a low-intensity “foot” of 3 to 5 ns length with
I = 10
12−10
13 W/cm
2, which sets the required compression adiabat of the imploding target. In such conditions laser imprinted perturbations were still observed for polystyrene (СH) targets with rms roughness < 30 Å, while hydrodynamic smoothing reduced them by an order of magnitude.
Among other foam applications, experiments at the 5-beam Shenguang III 3ω Nd: glass laser facility could be mentioned [
45] where a homogenous long-scale NCD plasma was produced by 4 laser beams with total energy 3.2 kJ in 1-ns pulses and intensity
I ≈ 8×10
14 W/cm
2 from uniformly irradiated foam with a density ~ 10 mg/cm
3. Interaction of the fifth delayed beam at intensity
I ~ 10
15 W/cm
2 with the plasma was investigated which modeled the LPI development in the ICF-scale conditions. Thick NCD foam targets were used by Romsej
et al. for direct laser acceleration (DLA) of electrons at relativistic intensity of 10
19 W/cm
2 in homogeneous plasma channel of sub-mm length preformed by a nanosecond laser pulse with intensity
I ≈ 5×10
13 W/cm
2 [
46,
47]. Long foam plasma gave a significant advantage in the DLA compared with a short-scale plasma produced in a conventional laser-foil interaction.
The present studies with low-density foam targets performed with a long-pulse GARPUN KrF laser at relatively low peak intensity ~ 10
12 W/cm
2 were motivated by our previous experiments [
48,
49] where in a specific two-dimensional (2D) geometry high-aspect-ratio capillary channels were obtained in semitransparent polymeric materials, e.g., polymethyl methacrylate (PMMA) and they revealed obvious features of the UV radiation waveguide. A direct electron acceleration in a self-produced, or preliminary drilled capillaries was observed up to a few hundred keV [
50], being associated with a longitudinal component of the electric field in a corrugated waveguide which retarded the light in phase with electrons [
51]. It is expected that the 2D hydrodynamics of low-density foam targets for 100-ns laser pulse would be rather different from the case of 1D geometry typical for the most laser-foam interaction studies [
22,
23,
24,
25,
26,
27,
28,
29,
30,
31,
32,
33,
34,
35,
36,
37,
38] carried out with ns-scale laser pulses. In addition, the most plastic materials have a steep rise in absorbance around KrF laser wavelength [
49], which should decrease the plasma formation time for foams. So, we believe that mm-scale plasma channels could be obtained with long KrF laser pulses.
4. PLDM hydrodynamics
Typical hydrodynamic picture of high-energy 100-ns pulse interaction with foam targets at GARPUN laser is illustrated in
Figure 8. At irradiation intensity
I ≈ 10
12 W/cm
2 the plasma produced from a CHO foam of the thickness
l = 200 μm and density
ρ = 20 mg/cm
3 expanded from a front side of the target towards incident radiation and from a back side in the laser beam direction with approximately equal velocities
v ≈ 75 km/s (a). A rapid volumetric absorption of radiation inside the foam determined the explosive nature of plasma formation. When the pulse energy
E (and, accordingly, the intensity) were reduced by 4.8 times, the plasma expansion velocity decreased down to
v ≈ 55 km/s (b). It means that the dependance of plasma front velocity on laser energy
formally coincides with Sedov–von Neumann–Taylor blast wave solution for the radius
R and velocity
v [
54]:
Here E is the energy release, ρ0 medium density, α coefficient depending on the adiabatic index γ; for γ=1.4 in air α ≈ 1.
Formula (1) is exactly valid for a strong instantaneous point massless explosion. It was also used to estimate energy load in foam explosion produced by a nanosecond pulse [
31]. In our case of a long 100-ns laser pulse, which was comparable with a hydrodynamic time scale, after a rapid foam explosion the produced plasma cloud quickly became transparent for UV radiation, and only a small fraction of the laser energy was released in the foam.
However, a finite time of the foam explosion and a finite focal spot size resulted in a different
R(
t) dependence (
Figure 9) compared with the formula (1). Only for the later time
t ≥35 ns the plasma blow-up velocity follows a relation
. By this moment the mass of surrounded air involved into the blast wave (for a residual pressure in the interaction chamber ~ 0.1 Torr) became comparable with the evaporated foam mass.
Measurements of the burn-through time performed with CHO foam of
l = 400 μm,
ρ = 20 mg/cm
3 and with an additional screen behind a target illustrated in
Figure 8 c confirm very fast foam explosion. The CHO foam became transparent with a delay Δ
t ≈ 10 ns after the beginning of the laser pulse. In the case of a thick SiO
2 aerogel with
l = 2.5 mm and
ρ = 100−150 mg/cm
3, the radiation passed through the plasma after ~ 30 ns. Thus, the measured burn-through rates are
vb ≈ 40 km/s in CHO foam and
vb ~ 80 km/s in SiO
2 aerogel. These measurements correspond to effective mass ablation rates
: 8×10
4 and ~10
6 g/cm
2‧s, respectively. A difference in
by an order of magnitude obviously originates from a tenfold difference in CHO foam and SiO
2 aerogel absorption coefficients for laser radiation (see above, section 3.2).
Ablation rates
in Al foil and graphite targets were measured in a similar layout earlier in the intensity range
I = (1−5)×10
12 W/cm
2 [
55]. Very high velocities were obtained for 100-ns pulses which exceeded by an order of magnitude the measured ones for nanosecond pulses. They were mostly caused by a hydrodynamic radial displacement of matter by a megabar-scale ablation pressure. An approximation formula for
was obtained:
where
is in [g/cm
2‧s] and
I in [W/cm
2].
In this regard, Al foils were used in present experiments to compare with foam targets. For peak radiation intensity
I ≈ 10
12 W/cm
2, burn-through times of 10−50 ns have been measured for foils of
l = 20−110 μm thicknesses (
Figure 10), which corresponds to the burn-through rate in aluminum
vb ≈ 2.2 km/s and effective mass ablation rate
≈ 6×10
5 g/cm
2‧s. These values coincide with our previous above-mentioned measurements. Plasma expansion velocity towards incident radiation was
v ≈ 80 km/s, i.e., approximately the same as for the foam targets with a volume absorption.
Figure 1.
Layout of transmittance measurements.
Figure 1.
Layout of transmittance measurements.
Figure 2.
Optical scheme for (a) studying the laser-target interaction and (b) measuring the burn-through time of targets.
Figure 2.
Optical scheme for (a) studying the laser-target interaction and (b) measuring the burn-through time of targets.
Figure 3.
Photos of foam targets made of (a) CH polymer in the form of a cylinder, (b) CHO film on the hoop, (c) SiO2 aerogel in the form of a parallelepiped.
Figure 3.
Photos of foam targets made of (a) CH polymer in the form of a cylinder, (b) CHO film on the hoop, (c) SiO2 aerogel in the form of a parallelepiped.
Figure 4.
Oscilloscope traces of incident (PD1) and transmitted (PD2) radiation for different foams and peak intensities: (1,2) CHO foam, I = 6×1010 W/cm2; (3,4) SiO2 aerogel, I = 4.5×1010 W/cm2; (5,6) CHO foam, I = 2.8×1010 W/cm2. PD2 signal (4) is multiplied by 5.
Figure 4.
Oscilloscope traces of incident (PD1) and transmitted (PD2) radiation for different foams and peak intensities: (1,2) CHO foam, I = 6×1010 W/cm2; (3,4) SiO2 aerogel, I = 4.5×1010 W/cm2; (5,6) CHO foam, I = 2.8×1010 W/cm2. PD2 signal (4) is multiplied by 5.
Figure 5.
Oscilloscope traces of incident (PD1) and transmitted (PD2) radiation for CH-film at peak intensities: (1,2) I = 6×1010 W/cm2; (3,4) I = 2.7×1010 W/cm2; (5,6) I = 1.3×1010 W/cm2. All PD2 signal were multiplied by 10.
Figure 5.
Oscilloscope traces of incident (PD1) and transmitted (PD2) radiation for CH-film at peak intensities: (1,2) I = 6×1010 W/cm2; (3,4) I = 2.7×1010 W/cm2; (5,6) I = 1.3×1010 W/cm2. All PD2 signal were multiplied by 10.
Figure 6.
A normalized laser pulse shape and PD2/PD1 ratio obtained for (1) CHO foam, I = 6×1010 W/cm2; (2) CHO foam, I = 2.8×1010 W/cm2; (3) SiO2 aerogel, I = 4.5×1010 W/cm2.
Figure 6.
A normalized laser pulse shape and PD2/PD1 ratio obtained for (1) CHO foam, I = 6×1010 W/cm2; (2) CHO foam, I = 2.8×1010 W/cm2; (3) SiO2 aerogel, I = 4.5×1010 W/cm2.
Figure 7.
A normalized laser pulse shape and PD2/PD1 ratio obtained for CH films at (1) I = 6×1010; (2) I = 2.7×1010; (3) I = 1.3×1010 W/cm2.
Figure 7.
A normalized laser pulse shape and PD2/PD1 ratio obtained for CH films at (1) I = 6×1010; (2) I = 2.7×1010; (3) I = 1.3×1010 W/cm2.
Figure 8.
Streak images of CHO foam with density ρ = 20 mg/cm3, different thicknesses l and peak irradiation intensities I: (a) l = 200 μm, I≈1012 W/cm2; (b) l = 200 μm and I≈0.21×1012 W/cm2; (c) l = 400 μm and I≈0.93×1012 W/cm2 with Al screen behind.
Figure 8.
Streak images of CHO foam with density ρ = 20 mg/cm3, different thicknesses l and peak irradiation intensities I: (a) l = 200 μm, I≈1012 W/cm2; (b) l = 200 μm and I≈0.21×1012 W/cm2; (c) l = 400 μm and I≈0.93×1012 W/cm2 with Al screen behind.
Figure 9.
Time evolution of the blast wave distances from the front R1 and from the back side R2 of the CHO foam (ρ = 20 mg/cm3, l = 200 μm, I≈1012 W/cm2).
Figure 9.
Time evolution of the blast wave distances from the front R1 and from the back side R2 of the CHO foam (ρ = 20 mg/cm3, l = 200 μm, I≈1012 W/cm2).
Figure 10.
(a) A burn-through measurements for Al foils: (a) a static target image with an additional screen; streak images for I≈1012 W/cm2 and different thicknesses l (b) l = 20, (c) 50 and (d) 110 μm.
Figure 10.
(a) A burn-through measurements for Al foils: (a) a static target image with an additional screen; streak images for I≈1012 W/cm2 and different thicknesses l (b) l = 20, (c) 50 and (d) 110 μm.