1. Introduction
Liquid crystals (LCs) represent a fascinating class of soft materials characterized by their fluidity combined with anisotropic properties, making them highly responsive to external fields and boundary conditions. This unique combination has led to widespread applications, particularly in display technologies, and has also spurred interest in fundamental research on the stability of their phases and topological structures [
1]. Among these structures, solitons in chiral nematic LCs have emerged as a significant area of study due to their rich topological properties and potential for novel technological applications [
2,
3]. Besides skyrmions, which are two-dimensional configurations, many other topological-protected structures were realized in experiments, including torons, hopfions, skyrmions and solitonic macromolecules. We will refer to torons as the three-dimensional elementary skyrmion terminating at two-point defects to satisfy the uniform surface boundary conditions and match the topologically nontrivial skyrmion tube with the uniform far-field background and reserve skyrmion to describe the two-dimensional midplane structure.
Solitons in liquid crystals are localized, non-singular distortions of the director field that exhibit robust particle-like behaviour and complex interactions. These structures are of particular interest due to their ability to be manipulated by external stimuli, such as electric fields, which can drive their motion and induce collective behaviour [
4,
5]. The study of soliton dynamics in LCs has provided insights into fundamental aspects of topology in soft matter and has highlighted their potential in advanced material applications, including reconfigurable optical devices and microfluidic systems [
4,
6,
7,
8,
9,
10,
11,
12,
13,
13].
While much of the research on LC torons has focused on their behaviour under uniform external fields, little is known under non-uniform conditions such as static colloids or other obstacles trapped in the LC matrix. Furthermore, only a handful of studies addressed the interaction between torons and mass flows [
14,
15,
16,
17] remaining an overlooked problem of relevance in various fields. Understanding the dynamical response of LC torons in non-uniform or heterogeneous media is relevant for practical applications, where flowing torons may encounter various types of obstacles, such as geometrically patterned substrates, dispersed colloidal particles or defects in the LC matrix. This response will significantly alter the torons’s initial trajectory, in addition to its shape and stability, potentially driving novel dynamical phenomena.
In the theoretical study of torons, three approaches are commonly used in the literature. The first approach involves the numerical solution of continuum equations resulting from the minimization of the elastic free energy, which is typically implemented using finite difference or finite volume methods [
4,
18,
19,
20]. This approach has focused either on the dynamic evolution of torons or on the stable configuration of static torons. The second approach is based on analytical studies of the continuum equations, under simplified conditions required to make the problems tractable [
21,
22]. This method often provides valuable insights into the toron behaviour in idealized situations. The third approach, a more recent development, uses particle-based modelling, where torons are treated as individual particles [
23]. Langevin dynamics is employed to simulate their motion, and potential functions for the toron interactions are inferred from experimental data or from simulations using the first method. In this study, we use the first approach combining it with the lattice Boltzmann method to simulate material flow, providing a comprehensive and versatile framework to study the interaction between topology and external mass flows that may be perturbed by an arbitrary array of obstacles.
In what follows, we study the flow of liquid crystal torons, driven by an external mass flow, around solid obstacles. The toron’s stability and trajectory are found to depend strongly on the impact parameter of the obstacle. When the impact parameter is less than m, the toron becomes unstable and disintegrates, in flows where torons would remain stable otherwise. However, when the impact parameter, is larger than m, the stability of the toron is preserved while the toron’s trajectory is deflected by an amount that decays exponentially with the impact parameter. Notably, the toron’s velocity is found to increase as it approaches the obstacles due to flow constriction. We have also examined the dynamics and stability of torons flowing around one and between two obstacles, providing additional insights into how multiple obstacles may influence the dynamics of flowing torons.
3. Results
We report the results of numerical simulations of a flowing toron driven by an external force, around a cylindrical pillar near its initial trajectory. The liquid crystal was initialized at rest, with alignment along the vertical direction, except at the toron, where we used the relaxed configuration obtained from the ansatz [
14]. The system dimensions were set to
, and the material parameters are listed in
Table 1. The pillar, with a radius of
m (or 5
), homeotropic anchoring and no-slip boundary was placed at
and
. The fluid was driven by an external body force of magnitude
m/s
2 (or
l.u.) in the
x direction.
As expected, the pillar distorts the velocity field and perturbs the toron initial trajectory, as shown in
Figure 1. In the midplane,
Figure 1(a), the toron shrinks slightly as it flows around the pillar but later recovers its original configuration. To confirm the toron’s stability post-pillar interaction, we relaxed the final configuration in
Figure 1 without the external force, confirming that it remains stable (not shown). The toron cross-section in
Figure 1(b) reveals that the toron becomes asymmetric in the direction of the flow, consistent with previous observations in Poiseuille-like flows without the pillar [
16]. The velocity field is perturbed by the toron, while the pillar introduces large velocity gradients in the flow field (
Figure 1(c)). In the cross-sectional view,
Figure 1(d), the flow exhibits a Poiseuille-like profile, except near the toron and the pillar.
The deflection of the initial trajectory of the toron depends on the impact parameter
h, as shown in
Figure 2. Trajectories are defected significantly when the impact parameter is less than cholesteric pitch. However, below a threshold,
m, or
P, in our simulations, the toron becomes unstable and disintegrates. The toron in Poiseuille flows already becomes unstable without the obstacle at higher speeds [
17] and here it occurs due to the local increase in the velocity field around the obstacle. When the toron collides directly with the pillar (
), it disintegrates before flowing around the obstacle. For small but non-zero values of
h, the toron flows around the pillar but later becomes unstable, as depicted in
Figure 3. The inset on the left of
Figure 2 depicts the deflection
of the toron initial trajectory as a function of the impact parameter,
h. As
h increases,
decays exponentially, reaching zero when the obstacle is sufficiently far from the toron so that the toron does not feel the change in the director field caused by the obstacle. The exponential decay is usually observed in the distortions in the liquid crystal orientation [
32]. The inset on the right shows the toron velocity as a function of position, where we note that a stable toron accelerates near the pillar, with its velocity increasing by about
before returning to its initial value, due to flow constriction by the pillar.
The free energy integrated over the entire volume, calculated using Eq.(
7), is plotted in
Figure 4 as a function of time for various impact parameters,
h. At small
h, the free energy rises sharply, reaching a peak when the toron loses stability and disintegrates. At larger impact parameters,
h, the toron remains stable, and the free energy stabilizes, with slight perturbations occurring as the toron flows around the pillar, particularly evident in the orange curve (
m) around
s.
Until now, we considered the flow of a toron around a single pillar. To explore the effects of multiple obstacles, we simulated the toron flow between two pillars, which act as a flow constriction (see
Figure 5). In this configuration, the toron accelerates by 44% as it flows between the pillars, as shown in
Figure 5(c). Similar to the single-pillar case, the toron becomes unstable at small values of
h. In our simulations, the toron remains stable for
m, which is almost twice the impact parameter required for toron stability in the single-pillar case. This is likely due to the toron’s size reduction when passing around the pillars, an effect that is amplified by the presence of two obstacles. Additionally, in this configuration, the toron does not deviate from its initial trajectory.
In addition to simulating the interaction between the toron and a cylindrical pillar with homeotropic anchoring, we investigated other obstacle geometries (not shown). For example, we replaced the pillar with a solid sphere, mimicking a colloid, and applied different anchoring conditions (both homeotropic and toron-like). However, no qualitative differences were observed. Thus, we conclude that the primary factor determining the flow of torons around obstacles, as well as their stability, appears to be the effect of the large velocity gradients introduced by the obstacles rather than their detailed form.